Monitoring rainwater and seaweed reveals the presence of 131I in southwest and central British Columbia, Canada following the Fukushima nuclear accident in Japan

Detailed analysis of 131I levels in rainwater and in three species of seaweed (Fucus distichus Linnaeus, Macrocystis pyrifera, and Pyropia fallax) collected in southwest British Columbia and Bella Bella, B.C., Canada was performed using gamma-ray spectroscopy following the Fukushima nuclear power plant accident on March 11, 2011. The maximum 131I activity was found to be 5.8(7) Bq/L in rainwater collected at the campus of Simon Fraser University in Burnaby, B.C. nine days after the accident. Concomitantly, the maximum observed activity in the brown seaweed Fucus distichus Linnaeus was observed to be 130(7) Bq/kg dry weight in samples collected in North Vancouver 11 days following the accident and 67(6) Bq/kg dry weight in samples collected from the Bamfield Marine Sciences Centre on Vancouver Island 17 days following the accident. The 131I activity in seaweed samples collected in southwest B.C. following the Fukushima accident was an order of magnitude less than what was observed in similar measurements performed in British Columbia following the Chernobyl accident. Iodine-131 activity in Fucus distichus Linnaeus remained detectable for 60 days following the accident and was detectable in each seaweed species collected. The Germanium Detector for Elemental Analysis and Radioactivity Studies (GEARS) was modeled using the GEANT4 software package and developed as an analytical tool by the Nuclear Science group in the Simon Fraser University Department of Chemistry for the purpose of these measurements.